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Using solubility difference to achieve surface phase separation in dimethylsiloxane-urea-urethane copolymers

  • George Mason University
  • Office of Naval Research
  • Naval Research Laboratory
  • SUNY Buffalo

Research output: Contribution to journalArticlepeer-review

19 Scopus citations

Abstract

Effects of the casting solvent on the surface compositions of a series of polydimethylsiloxane (PDMS)-urethane-urea copolymers were investigated. The solvent pair investigated was tetrahydrofuran (THF) and mineral spirits (MS). Factors that determine solubility of a copolymer in a mixture of THF and MS include the solvent composition and the ratio between the sizes of the soft and the hard segments. The effectiveness of using mixed solvent to enhance surface PDMS enrichment varies with the copolymer composition. The benefits are maximized when the average molecular weight of the PDMS segments is 10,000.

Original languageEnglish
Pages (from-to)277-279
Number of pages3
JournalJournal of Colloid and Interface Science
Volume176
Issue number1
DOIs
StatePublished - Dec 1 1995

Keywords

  • PDMS-PU copolymer
  • Selective precipitation
  • Solvent effect
  • Surface phase separation

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