Abstract
When an electron is transferred to C60, the electron-lattice interaction results in a distortion of the bond structure and a polaronlike state is formed. By solving the dynamical equations of molecules in a C60 cage, the time-dependent changes of the bond lengths are obtained. We find that the relaxation time to form a polaron is about 0.3 ps, and is consistent with the experimental results. The implication of this ultrafast evolution, with comparison to the soliton-antisoliton mechanism, is discussed.
| Original language | English |
|---|---|
| Pages (from-to) | 11976-11980 |
| Number of pages | 5 |
| Journal | Physical Review B-Condensed Matter |
| Volume | 50 |
| Issue number | 16 |
| DOIs | |
| State | Published - 1994 |
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