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Metal-insulator transition in surface-doped VO2 nanowires at liquid helium temperature

  • Seok Hwang Yun
  • , Jeong Min Baik
  • , Jong E. Han
  • , Muhammad Atif Khan
  • , Sun Jin Yun
  • , Gil Ho Kim
  • Sungkyunkwan University
  • Korea Research Institute of Chemical Technology

Research output: Contribution to journalArticlepeer-review

Abstract

The metal-insulator transition (MIT) in VO2 nanowire devices, driven by electric field-induced nonequilibrium effects, is observed at liquid helium temperature. This unusually low transition temperature is achieved by surface doping VO2 nanowires with gold nanoparticles (NPs). The presence of gold NPs may promote percolative conduction pathways, enhance electronic inhomogeneity, or alter lattice–electron coupling. These effects collectively enable a smoother MIT at a lower electric field compared to pristine VO2 nanowires. An empirical model is used to distinguish Joule heating from electric field contributions, confirming the dominance of nonequilibrium electric field effects. Repeated voltage sweeps further reveal hysteresis and current variations, providing insights into carrier dynamics and correlated electron behavior introduced by NP decoration. These findings advance understanding of the MIT mechanism in VO2 and emphasize the role of surface modifications in tailoring phase transitions at cryogenic temperatures.

Original languageEnglish
Article number116479
JournalPhysica E: Low-Dimensional Systems and Nanostructures
Volume179
DOIs
StatePublished - Apr 1 2026

Keywords

  • Au nanoparticles
  • Dielectrophoresis
  • Metal-to-insulator transition
  • Mott and peierls transition
  • VO nanowires

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