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Frequency dependence of two-photon resonance and damping in polymers

  • X. Sun
  • , K. Nasu
  • , C. Wu
  • , L. Li
  • , D. L. Lin
  • , T. F. George
  • Fudan University
  • Institute for Molecular Sciences
  • Abdus Salam International Centre for Theoretical Physics
  • SUNY Buffalo

Research output: Contribution to journalArticlepeer-review

1 Scopus citations

Abstract

For the two-photon resonance in the spectrum of third-harmonic generation (THG) of trans-polyacetylene, the existing theories can only qualitatively, rather than quantitatively, accord with the experimental data. In this paper a damping mechanism is proposed. It shows that once the excitation-dependent damping is taken into account, the whole experimental spectrum of the THG can be quantitatively interpreted by our theory.

Original languageEnglish
Pages (from-to)141-145
Number of pages5
JournalSynthetic Metals
Volume49
Issue number1-3
DOIs
StatePublished - Aug 1 1992

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