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Feasibility study on pressure swing sorption for removing H2S from natural gas

  • Li Zhou
  • , Miao Yu
  • , Limei Zhong
  • , Yaping Zhou
  • School of Chemical Engineering and Technology
  • Tianjin University

Research output: Contribution to journalArticlepeer-review

24 Scopus citations

Abstract

The possibility of removing H2S from natural gas by applying a pressure swing sorption (PSS) process was experimentally proven. The key technique of the PSS process relies on using a special type of sorbent where solid grains were coated by a layer of liquid. It was shown that the solubility of H2S in the layer of liquid enlarged the concentration of H2S at the solid surface and, hence enhanced the adsorption of H2S on adsorbent. The solubility of H2S is very sensitive to the partial pressure above the layer of liquid, therefore, the saturated sorbent could be easily regenerated by sweeping the bed of sorbent with nitrogen at ambient temperature and pressure. The sorption capacity as well as the coated sorbent was stable during the operation cycles of sorption/desorption. The new PSS technology of sweetening natural gas is advantageous over the prevailing technologies of today in that both savings of investment and energy cost could be expected.

Original languageEnglish
Pages (from-to)2401-2406
Number of pages6
JournalChemical Engineering Science
Volume59
Issue number12
DOIs
StatePublished - Jun 2004

Keywords

  • Natural gas sweetening
  • NMP
  • Pressure swing sorption
  • Silica gel

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