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Effect of surface oxygen groups on the irreversible adsorption of organic vapors

  • Masud Jahandar Lashaki
  • , John D. Atkinson
  • , Zaher Hashisho
  • , John H. Philips
  • , James E. Anderson
  • , Mark Nichols
  • University of Alberta
  • Ford Motor Company

Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

Abstract

The effect of activated carbon's oxygen functional groups on the irreversible adsorption of organic vapors emitted from automotive painting operations was investigated. Microporous beaded activated carbon (BAC) was treated with H2 to remove oxygen groups or treated with nitric acid to add acidic oxygen groups. No significant change in mass balance cumulative heel was observed. Stronger physisorption was noted for heat-treated and H2-treated BAC. A combination of weak physisorption and strong chemisorptions resulted to heel formation on nitric acid-treated BAC. BET surface area and pore volumes of the adsorbents decreased due to heel accumulation, and the largest reduction occurred for nitric acid-treated BAC. Pore size distributions showed that narrow micropores have a major role in the accumulation of adsorbates in heat-treated and H2-treated BAC, while larger micropores were responsible for heel formation in nitric acid-treated BAC. This is an abstract of a paper presented at the AWMA's 107th Annual Conference & Exhibition (Long Beach, CA 6/24-27/2014).

Original languageEnglish
Title of host publication107th Air and Waste Management Association Annual Conference and Exhibition, ACE 2014
PublisherAir and Waste Management Association
Pages2288-2300
Number of pages13
ISBN (Electronic)9781634397322
StatePublished - 2014

Publication series

NameProceedings of the Air and Waste Management Association's Annual Conference and Exhibition, AWMA
Volume3
ISSN (Print)1052-6102

Keywords

  • Activated carbon
  • Irreversible adsorption
  • Organic vapors
  • Surface oxygen groups

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